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From Biology-Online Dictionary
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1. To insert in a roll; to register or enter in a list or catalogue or on rolls of court; hence, to record; to insert in records; to leave in writing; as, to enroll men for service; to enroll a decree or a law; also, reflexively, to enlist.

2. To envelop; to inwrap; to involve.

alternative forms: enrol.

Origin: f. Enroler; pref. En- (L. In) _ role = roll or register.